It took Moore till SWLM to deliver his best Bond but SC did in his 2nd, while his GF & TB performances are great, his FRWL is devoid of too many gadgets save the practical attache case, the way it's incorporated into the train fight is simply genius and still my all time stand alone Bond moment.
I think that Connery was very lucky to get a first-class Bond film with his 2nd outing, whereas Moore had to wait until his third film - TSWLM - to strike gold.